Scalable production of nuclear battery alpha emitters using fusion neutrons
J. F. Parisi
Nuclear batteries powered by alpha decay have been deployed successfully for over 60 years, on a worldwide $^{238}$Pu supply of kilograms per year. We show that the 14 MeV neutrons of a single deuterium-tritium fusion plant can produce alpha emitter battery fuels up to tons per year, in three classes: fuels with completely new production pathways ($^{236}$Pu, $^{227}$Ac, $^{210}$Pb), fuels previously proposed whose scarce feedstock the same pathways now breed at scale ($^{232}$U, $^{228}$Th), and the established $^{238}$Pu. OpenMC simulations of actinide channels in a tokamak blanket give, per GW yr of fusion: 11 to 57 kg of $^{236}$Pu, whose chain releases 18 GJ per gram over a century, ending at stable $^{208}$Pb, plus up to 5.2 t of co-product $^{238}$Pu; up to 1.4 t of $^{231}$Pa from thorium, and, from channel with $^{231}$Pa feedstock, up to $\sim$15 t of $^{232}$U or $\sim$122 kg of $^{210}$Pb, with $^{227}$Ac produced at 21 g/yr per tonne of $^{231}$Pa. Neutron capture also upgrades $^{241}$Am to a $^{242}$Cm/$^{242m}$Am/$^{241}$Am/$^{238}$Pu blend with up to 10 times higher power density. The same $^{236}$Pu and $^{232}$U also serve as proliferation safeguards: the $^{237}$Np, $^{232}$Th, and $^{231}$Pa channel products are self-protecting, the plutonium by $^{236}$Pu and $^{238}$Pu decay heat and the 2.6 MeV gammas from $^{208}$Tl content, and similarly the uranium from its $^{232}$U. Many of these fuels ($^{236}$Pu, $^{232}$U, $^{228}$Th, $^{227}$Ac) have an order of magnitude higher power and energy density than current alpha emitters, and at human spaceflight-relevant doses the $^{227}$Ac and $^{210}$Pb chains need less shield mass than $^{238}$Pu or $^{241}$Am above a few hundred watts. Fusion neutrons could therefore enable nuclear batteries at the kilowatt to megawatt scale and unlock new possibilities for power sources requiring exceptionally high energy density.
